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Data for: Polariton condensation in a microcavity using a highly-stable molecular dye

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Version 2 2022-10-04, 08:00
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posted on 2022-10-04, 08:00 authored by Kirsty McGhee, Rahul JayaprakashRahul Jayaprakash, Kyriacos Georgiou, Stephanie BurgStephanie Burg, David LidzeyDavid Lidzey

 We have fabricated dielectric microcavities containing the molecular dye 1,4-bis[2-[4-[N,N-di(p-tolyl)amino]phenyl]vinyl]benzene (DPAVB) dispersed in a transparent polymer matrix. We show that despite the relatively broad absorption linewidth of the DPAVB, the cavities enter the strong coupling regime. We use <330 ps pulses at 355 nm from a Nd:YAG laser to generate amplified spontaneous emission from control films and polariton condensation from the strongly-coupled microcavity in air and at room temperature. Here, polariton condensation is observed at an excitation threshold of 215 μJ cm−2. Significantly, we show that the DPAVB dye has a very high degree of photostability, with polariton condensation still observed from the cavity after 37 000 excitation pulses, showing promise for its use in practical polaritonic devices. 

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Hybrid Polaritonics

Engineering and Physical Sciences Research Council

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DTP 2018-19 University of Sheffield

Engineering and Physical Sciences Research Council

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